Transient magnetic resonance of a photoexcited quartet state |
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Authors: | G. Kothe S.S. Kim S.I. Weissman |
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Affiliation: | Institute of Physical Chemistry, University of Freiburg, Freiburg, Germany;Department of Chemistry, Washington University, St. Louis, Missouri, USA |
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Abstract: | Wide-band detection following pulsed laser excitation of the decacyclene anion has yielded transient election paramagnetic resonance signals which we assign to an excited quartet state. The spin-spin coupling constant D and the path of intersystem crossing from doublet to quartet have been determined. |
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