Intramolecular dynamics: time evolution of superposition states in the regular and irregular spectrum |
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| Authors: | Paul Brumer Moshe Shapiro |
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| Institution: | Department of Chemistry University of Toronto, Toronto Ontario, Canada;Department of Chemical Physics, Weizmann Institute of Science Rehovot, Israel |
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| Abstract: | The time evolution of wavefunctions ψ(t) is compared in two systems, one with a regular energy spectrum and one with an irregular spectrum. The behavior of P(t) = {|ψ(O)|ψ(y]}|2 is found to be the same in both systems, P(t) decay is insensitive to the coupling between the degrees of freedom. |
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