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Nonlinear optical and XPS properties of Au and Ag nanometer-size particle-doped alumina films prepared by the sol–gel method
Authors:T Ishizaka  S Muto and Y Kurokawa
Institution:

a Department of Material Chemistry, Graduate School of Engineering, Tohoku University, Aramaki, Aoba-ku, Sendai 980-8579, Japan

b Department of Electrical Engineering and Computer Science, Faculty of Engineering, Yamanashi University, Takeda, Kofu 400-8511, Japan

Abstract:Au and Ag nanometer-size particle-doped alumina films were prepared by the aqueous sol–gel method. Their XPS and third-order nonlinear optical properties were examined. The XPS results gave evidence of an interaction between Au and alumina. Third-order susceptibilities, χ(3) and χ(3)/greek small letter alpha obtained by degenerate four-wave mixing method were in the order of 10?8 esu and 10?10 esu.cm for doped films, respectively.
Keywords:Nonlinear optics  Alumina  Nanometer-size particle  Noble metal
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