The AsO radical detected by infrared laser magnetic resonance |
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Authors: | H Uehara |
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Institution: | Department of Chemistry, Kansas State University, Manhattan, Kansas 66506, USA;Department of Biological Sciences and Center for Laser Studies, University of Southern California, Los Angeles, California 90007, USA |
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Abstract: | The Pauli master equation for intramolecular vibrational relaxation and the heat bath feedback Bloch equations for radiative pumping of polyatomic molecules can be derived by replacing the standard assumption of random matrix element coupling between zero-order vibrational states by an assumption that relaxation is governed by restricted quantum exchange. |
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