General theory of vibrational mode mixing and frequency shifts in resonance raman scattering |
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Authors: | D.L. Tonks J.B. Page |
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Affiliation: | Department of Physics, Arizona State University, Tempe, Arizona 85281, USA |
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Abstract: | A general formalism is given for treating vibrational mode mixing, frequency shifts, and atomic equilibrium position shifts under electronic excitation in resonance Raman scattering. The theory is exact for first-order scattering at T = 0 K for all linear and quadratic electron-phonon coupling strengths. Numerical results illustrating mode mixing are presented. |
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Keywords: | Present address: Chemical Research Institute of Nonaqueous Solutions Tohoku University Sendai 980 Japan. |
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