Unusual magneto-optical phenomenon reveals low energy spin dispersion in the spin-1 anisotropic Heisenberg antiferromagnetic chain system NiCl2-4SC(NH2)_{2} |
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Authors: | Cox S McDonald R D Armanious M Sengupta P Paduan-Filho A |
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Institution: | National High Magnetic Field Laboratory, Los Alamos National Laboratory, MS-E536, Los Alamos, New Mexico 87545, USA. |
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Abstract: | Electron paramagnetic resonance measurements of NiCl2-4SC(NH2)_{2} reveal the low-energy spin dispersion, including a magnetic-field interval in which the two-magnon continuum is within k_{B}T of the ground state, allowing a continuum of excitations over a range of k states, rather than only the k=0 single-magnon excitations. This produces a novel Y shape in the frequency-field EPR spectrum measured at T > or = 1.5 K. Since the interchain coupling J_{ perpendicular}
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