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Spectroscopy of Single Dibenzoterrylene Molecules in para‐Dichlorobenzene
Authors:Nico R Verhart  Dr Mathias Müller  Prof Dr Michel Orrit
Institution:1. Huygens-Kamerlingh Onnes Laboratorium, Leiden University, The Netherlands;2. Isabellenhütte Heusler GmbH & Co KG., Dillenburg, Germany
Abstract:We study single dibenzoterrylene (DBT) molecules embedded in 1,4‐dichlorobenzene (para‐dichlorobenzene, pDCB) at 1.2 K. Due to the relatively low melting point of pDCB (53 °C), this host‐guest system can be easily prepared from the molten phase. Narrow linewidths, stable molecular lines and high saturation count rates of single DBT molecules were observed. For this reason, we consider this host‐guest system a promising candidate for the study of interactions of single molecules with other small objects such as waveguides or nanoparticles.
Keywords:excitation  fluorescence  high-resolution spectroscopy  single-molecule optics  spectral diffusion
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