Photon echo and stimulated photon echo study of various collisional-relaxation channels |
| |
Authors: | N N Rubtsova L S Vasilenko E B Khvorostov |
| |
Institution: | (1) Institute of Semiconductor Physics, Siberian Branch of the Russian Academy of Sciences, 630090 Novosibirsk, Russia |
| |
Abstract: | Collisional relaxation in SF6 gas and its mixtures with He and Xe is studied by photon echo and stimulated photon echo methods from the standpoint of the
possibility of identifying the contributions of different types of collisions. The nonexponential nature of the kinetic curve
of the photon echo is clearly observed for pure SF6, it is weaker in the mixture SF6+Xe, and it is virtually completely absent for high degrees of dilution of SF6 with helium. These features can be explained on the basis of estimates, made from experimental data, of the critical delay
between the exciting pulses (for which the nonexponential behavior should be most strongly manifested). In pure SF6 it is possible to distinguish the contribution of the inelastic channel (rotational relaxation) and the contribution of weak
collisions. To distinguish successfully the relaxation channels in mixtures with buffer gases a heavier buffer gas and a much
better time resolution must be used. It is shown that data obtained on the orientation and alignment relaxation rates by the
stimulated photon echo method can serve as an upper limit for the rates of inelastic processes which cannot be measured by
the photon echo method. The combined use of photon echo and stimulated photon echo methods made it possible to obtain data
on the cross sections for elastic and inelastic scattering of the collisional pairs SF6–SF6, SF6–Xe, and SF6–He.
Zh. éksp. Teor. Fiz. 116, 47–56 (July 1999) |
| |
Keywords: | |
本文献已被 SpringerLink 等数据库收录! |
|