Theory of two-photon absorption and emission second-order saturation effect |
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Authors: | O. Kafri S. Kimel |
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Affiliation: | School of Applied Science and Technology, Hebrew University, Jerusalem, Israel;Department of Chemistry, Technion - Israel Institute of Technology, Haifa, Israel |
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Abstract: | A simplified theory of small-signal two-photon absorption is developed, based on the solution of rate equations involving an infinitely short-living intimediate state. It is shown that in a first approximation this theory leads to results identical to those obtained using second-order perturbation techniques. Moreover, the present approach leads to a built-in saturation effect at high intensities depending on the parameters of the laser and of the absorbing medium. An analysis expression is given for the intensity dependent saturation. |
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