Mott gap excitations in twin-free YBa2Cu3O7-delta (Tc=93 K) studied by resonant inelastic x-ray scattering |
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Authors: | Ishii K Tsutsui K Endoh Y Tohyama T Kuzushita K Inami T Ohwada K Maekawa S Masui T Tajima S Murakami Y Mizuki J |
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Affiliation: | Synchrotron Radiation Research Center, Japan Atomic Energy Research Institute, Hyogo 679-5148, Japan. kenji@spring8.or.jp |
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Abstract: | Mott gap excitations in the optimally doped high-T(c) superconductor YBa(2)Cu(3)O(7-delta) (T(c)=93 K) have been studied by the resonant inelastic x-ray scattering method. Anisotropic spectra in the ab plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the b* direction, while the excitation from the CuO2 plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculations based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO2 plane site. |
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