Synthetic studies toward FR182877. Remarkable solvent effect in the vinylogous morita-baylis-hillman cyclization |
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| Authors: | Methot Joey L Roush William R |
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| Affiliation: | Department of Chemistry, University of Michigan, Ann Arbor, Michigan 48109, USA. |
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| Abstract: | [reaction: see text]. The intramolecular vinylogous Morita-Baylis-Hillman reaction was explored to access the central cyclopentane ring of FR182877. The reaction manifold and product distribution is strikingly solvent and substrate dependent. |
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