Expedient Route to the functionalized calyciphylline A-type skeleton via a Michael addition-RCM strategy |
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| Authors: | Sladojevich Filippo Michaelides Iacovos N Benjamin Darses Ward John W Dixon Darren J |
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| Institution: | Chemistry Research Laboratory, Department of Chemistry, University of Oxford, Mansfield Road, Oxford, OX1 3TA, UK. |
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| Abstract: | An efficient, robust, and scalable strategy to access the functionalized core of calyciphylline A-type alkaloids has been developed starting from commercially available 3-methylanisole. Key features of this approach are an intramolecular Michael addition/allylation sequence and a ring-closing metathesis step. |
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