Effects of anharmonic splitting upon collisionless multiple-photon laser excitation of SF6 |
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| Authors: | C.D. Cantrell H.W. Galbraith |
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| Affiliation: | Theoretical Division, University of California, Los Alamos Scientific Laboratory, Los Alamos, New Mexico 87545, USA |
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| Abstract: | Qualitative agreement of the dependence of molecular excitation upon laser frequency, between non-perturbative quantum-mechanical calculations and experimental measurements of the collisionless multiple-photon excitation of a few vibrational quanta in SF6 by a CO2 laser, results when anharmonic splitting of the vibrational energy levels is taken into account. |
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