High uptakes of CO2 and CH4 in mesoporous metal-organic frameworks MIL-100 and MIL-101 |
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| Authors: | Llewellyn Philip L Bourrelly Sandrine Serre Christian Vimont Alexandre Daturi Marco Hamon Lomig De Weireld Guy Chang Jong-San Hong Do-Young Kyu Hwang Young Hwa Jhung Sung Férey Gérard |
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| Affiliation: | Laboratoire Chimie Provence, Université de Provence - CNRS (UMR 6264), Centre de St Jér?me, 13397 Marseille Cedex 20, France. philip.llewellyn@univ-provence.fr |
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| Abstract: | Mesoporous MOFs MIL-100 and MIL-101 adsorb huge amounts of CO2 and CH4. Characterization was performed using both manometry and gravimetry in different laboratories for isotherms coupled with microcalorimetry and FTIR to specify the gas-solid interactions. In particular, the uptake of carbon dioxide in MIL-101 has been shown to occur with a record capacity of 40 mmol g(-1) or 390 cm3STP cm(-3) at 5 MPa and 303 K. |
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