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Characterisation of gas-liquid two-phase flow in minichannels with co-flowing fluid injection inside the channel,part II: gas bubble and liquid slug lengths,film thickness,and void fraction within Taylor flow
Institution:1. State Key Laboratory of Chemical Engineering, Collaborative Innovation Center of Chemical Science and Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, PR China;2. Laboratory of Reactions and Process Engineering, University of Lorraine, CNRS, 1, rue Grandville, BP 20451, 54001 Nancy cedex, France;1. Université de Toulouse, INSA, LISBP, 135 Av. de Rangueil, F-31077 Toulouse, France;2. INRA UMR792, Ingénierie des Systèmes Biologiques et des Procédés, F-31400 Toulouse, France;3. CNRS UMR 5504, Ingénierie des Systèmes Biologiques et des Procédés, F-31400 Toulouse, France;4. Université de Toulouse, INPT, LGC, 4 Allée Emile Monso, F-BP 84234, 31432 Toulouse, France;5. CNRS UMR 5503, Laboratoire de Génie Chimique, F-31432 Toulouse, France;6. Fédération de Recherche FERMAT, CNRS, Toulouse, F-31400 Toulouse, France
Abstract:Current research proofs the potential of apparatuses containing minichannel flow structures to intensify gas-liquid-solid contacting processes. The excellent heat and mass transfer in these devices as well as a sharp RTD mainly result from the Taylor flow regime. A proper design of corresponding contactors requires precise information on the provided interfacial areas. However, the characterisation of gas-liquid Taylor flow with industrially relevant fluids at elevated pressure and created by capillary injection devices gained little attention so far.This work analyses adiabatic gas-liquid Taylor flow in a square minichannel of 1.0 mm hydraulic diameter using water, water-glycerol, or water-ethanol mixtures as liquid phase and hydrogen or nitrogen as gas phase to cover a broad range of material parameters. In the mixing zone located within the flow channel, gas was injected into the co-flowing liquid by so-called capillary injectors with variable inner diameter (0.184, 0.317, 0.490 mm).Two different bubble forming mechanisms were identified leading to a complex interaction between physical properties of the fluids, geometrical parameters and the observed gas bubble and liquid slug lengths. According to the Pi-theorem, these lengths were affected by 6 dimensionless groups, namely (uG,s/ uL,s), ReL, WeL, (dIn,CI/ dh), (dOu,CI / dh), and Θ*. Based on more than 370 experimental data, novel correlations to predict gas bubble and liquid slug lengths were developed.
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