| 大气氧谱带的实验研究 |
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| 引用本文： | 宁利新,程平,王鸿梅,曹德兆,储焰南.大气氧谱带的实验研究[J].化学物理学报(中文版),2001,14(2):141-146. |
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| 作者姓名： | 宁利新 程平 王鸿梅 曹德兆 储焰南 |
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| 作者单位： | 中国科学院安徽光机所
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| 摘 要： | 利用流动余辉装置，首次报道了金属镍表面催化基态氧原子O(3P)复合从而获得大气氧谱带O2 （b1Σg+→X3Σg-）的(0,0)电子跃迁光谱。并且对反应管壁去激活O2 (b1Σg+)的动力学过程进行了分析，间接证实了O2 (b1Σg+)的浓度在反应管中是非稳态的变化过程。最后对O2 (b1Σg+)的形成机理进行了简单的讨论。
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| 关 键 词： | 流动余辉 大气氧谱带 能量转移 |
Experimental Research on Atmospheric Oxygen Band |
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| Ning Lixin,Cheng Ping,Wang Hongmei,Cao Dezao,Chu Yannan.Experimental Research on Atmospheric Oxygen Band[J].化学物理学报(中文版),2001,14(2):141-146. |
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| Authors: | Ning Lixin Cheng Ping Wang Hongmei Cao Dezao Chu Yannan |
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| Abstract: | Using the Ni surface-catalyzed excitation method, we obtained the (0,0) electronic transition spectra of atmospheric oxygen band (b1Σg+→X3Σg-) from the recombination of ground state oxygen atoms O(3P) in flowing afterglow apparatus. We experimentally analysed the kinetic process of deactivation of O2(b) by the wall, which indirectly proved that the concentration of O2(b)changed in a nonsteady-state way in the flowing tube. Meanwhile, the formation mechanism of O2 (b) was simply discussed. |
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| Keywords: | Flowing afterglow Atmospheric oxygen band Energy transfer |
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