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Large coupled magnetoresponses in EuNbO2N
Authors:Jorge A Belén  Oró-Solé Judith  Bea Ana M  Mufti Nandang  Palstra Thomas T M  Rodgers Jennifer A  Attfield J Paul  Fuertes Amparo
Institution:Institut de Ciència de Materials de Barcelona (C.S.I.C.), Campus U.A.B., 08193 Bellaterra, Spain.
Abstract:We have explored a new strategy to discover materials with large resistive or capacitive responses to magnetic fields by synthesizing EuMO2N (M = Nb, Ta) perovskites that combine ferromagnetic order of S = 7/2 Eu2+ spins with possible off-center distortions of the d0 M5+ cations enhanced by covalent bonding to N. EuNbO2N shows colossal magnetoresistances at low temperatures and a giant magnetocapacitance. However, the latter response originates from a microstructural effect rather than an intrinsic multiferroism.
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