Broadening and shift of the spectral line centers of a molecule upon strong vibrational excitation |
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| Authors: | A. D. Bykov D. S. Emel’yanov V. N. Stroinova |
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| Affiliation: | 1.V. E. Zuev Institute of Atmospheric Optics of the Siberian Branch of the Russian Academy of Sciences,Tomsk,Russia;2.National Research Tomsk Polytechnic University,Tomsk,Russia |
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| Abstract: | Half-widths and shifts of the line centers of the excited CO molecule caused by transitions between highly excited rovibrational states are calculated. Strong intramolecular effects caused by vibrational excitation are considered in the calculations. It is revealed that the vibrational dependence of the line broadening and shift coefficients is nonmonotonic, and the coefficients can change several times. |
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