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Interfacial Design of Dendrite‐Free Zinc Anodes for Aqueous Zinc‐Ion Batteries
Authors:Qi Zhang  Jingyi Luan  Yougen Tang  Xiaobo Ji  Haiyan Wang
Abstract:Aqueous zinc‐ion batteries have rapidly developed recently as promising energy storage devices in large‐scale energy storage systems owing to their low cost and high safety. Research on suppressing zinc dendrite growth has meanwhile attracted widespread attention to improve the lifespan and reversibility of batteries. Herein, design methods for dendrite‐free zinc anodes and their internal mechanisms are reviewed from the perspective of optimizing the host–zinc interface and the zinc–electrolyte interface. Furthermore, a design strategy is proposed to homogenize zinc deposition by regulating the interfacial electric field and ion distribution during zinc nucleation and growth. This Minireview can offer potential directions for the rational design of dendrite‐free zinc anodes employed in aqueous zinc‐ion batteries.
Keywords:coulombic efficiency  interface design  zinc anodes  zinc dendrites  zinc-ion batteries
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