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Disparities between experimental and environmental conditions: Research steps toward making electrochemical water treatment a reality
Authors:Sergi Garcia-Segura  Alec Brockway Nienhauser  Ana S Fajardo  Rishabh Bansal  Christian L Conrad  John D Fortner  Mariana Marcos-Hernández  Tanya Rogers  Dino Villagran  Michael S Wong  Paul Westerhoff
Institution:1. Nanosystems Engineering Research Center for Nanotechnology-Enabled Water Treatment, USA;2. School of Sustainable Engineering and the Built Environment, Arizona State University, Tempe, AZ, 85287, USA;3. Sorbonne Université, CNRS, Laboratoire Interfaces et Systèmes Electrochimiques (LISE), 4 Place Jussieu, Paris, F-75005, France;4. Department of Chemical and Biomolecular Engineering, Rice University, Houston, TX, 77005, USA;5. Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, 06520, USA;6. Department of Chemistry and Biochemistry, The University of Texas at El Paso, El Paso, TX, 79968, USA
Abstract:Electrochemical water treatment is one of the key topics of environmental electrochemistry. Identifying electrocatalytic materials capable of electrogenerating high oxidant species in situ seems to have catalyzed researchers’ interest in these processes. While most studies have focused on ideal lab-made solutions, translation to higher technology readiness levels and commercialization requires reframing research questions in context of real water matrices. In this current opinion, we discuss disconnects that may occur when focusing on synthetic solution treatment rather than on real waters. Future research can fill the gaps identified herein, thus facilitating application of electrochemical water treatment technologies.
Keywords:Electrocatalytic water treatment  Electrochemical advanced reduction processes  Electrochemical advanced oxidation processes  Boron-doped diamond electrode  Persistent organic pollutants  Oxyanions
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