NMR dynamics in disordered magnets

The excitation dynamics of site diluted magnets can be described at low energies (long length scales) by magnons, and above a crossover frequency, ω_c, (short length scales) by fractons. The density of fracton states is given by , where is the fracton dimensionality. Dilution gives rise to a characteristic length ξ∝(p−p _c)^ν, wherep _c is the critical concentration for (magnetic) percolation. The crossover frequency ω_c is proportional to ξ^-1[1+(θ/2)], where θ is the rate at which the diffusion constant decays with distance for diffusion on an equivalent network. A fractal dimensionD describes the density of magnetic sites on the infinite network, and . For percolating networks, for all dimensions ≥2. Neutron scattering structure factor measurements by Uemura and Birgeneau compare well with calculations using fracton concepts. Magnons are extended at low energies, while the fracton states are geometrically localized, with a wave function envelope proportional to exp . Here, is the fracton length scale at frequency ω. The exponentd _ϕ lies between 1 andd _min, the chemical length index (of the order of 1.6 in three dimensions). The localization of the magnetic excitations causes a spread in the NMR relaxation rates. A given nuclear moment will experience only a limited set of fracton excitations, resulting in an overall non-exponential decay of the NMR relaxation signal. When strong cross-relaxation is present, the relaxation will be exponential, but the temperature dependence will be strongly altered from the concentrated result.