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The challenges in reliable determination of degradation rates and lifetime in polymer electrolyte membrane fuel cells
Authors:Qian Zhang  Corinna Harms  Jens Mitzel  Pawel Gazdzicki  K. Andreas Friedrich
Affiliation:1. German Aerospace Center (DLR), Institute of Engineering Thermodynamics, Pfaffenwaldring 38-40, 70569 Stuttgart, Germany;2. German Aerospace Center (DLR), Institute of Engineering Thermodynamics, Carl-von-Ossietzky-Str. 15, 26129 Oldenburg, Germany;3. University of Stuttgart, Institute of Building Energetics, Thermal Engineering and Energy Storage (IGTE), Pfaffenwaldring 31, 70569 Stuttgart, Germany
Abstract:The durability of polymer electrolyte membrane fuel cells (PEMFCs) needs to be further improved to cope with application requirements and economic competitiveness. This article highlights the challenges in the reliable determination of degradation rates and lifetime. The reliable evaluation of performance degradation rates is fundamental to quantify and benchmark durability and to allow comparisons between PEMFC durability tests performed using different materials or in different laboratories. The use of efficient recovery procedures enables the discrimination of reversible and irreversible voltage losses and facilitates the understanding of recovery mechanisms. In the end, recent contributions about lifetime diagnoses and prediction are presented, which are promising to be implemented in PEMFC applications.
Keywords:Polymer electrolyte membrane fuel cells  Reversible degradation  Irreversible degradation  Recovery procedure  Durability evaluation
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