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Magnetic tunneling told to ignorants by two ignorants
Authors:J Villain  A Fort
Institution:(1) Centre de Recherches sur les Très basses températures, CNRS, BP 166, 38042 Grenoble Cedex 9, France, FR;(2) Département de Recherche Fondamentale sur la Matière Condensée, Commissariat à l'énergie Atomique, 17 avenue des Martyrs, 38054 Grenoble Cedex 9, France, FR;(3) Dipartimento di fisica, Università di Firenze, Istituto Nazionale di Fisica della Materia, Unità di Firenze, Largo Enrico Fermi 2, 50125 Firenze, Italy, IT
Abstract:Magnetic tunneling of a large spin subject to the Hamiltonian is investigated by elementary methods for weak fields H. In zero field (H=0) the tunnel frequency in the ground state is found to be equal to 0pt] multiplied by a quantity whose variation with s is slower than exponential. This result coincides with that of path integral methods #!schi!#]. For the values of the longitudinal field which allow tunneling, the tunnel frequency is shown to vanish when H y =0 for certain “diabolic" values of 0pt] , in qualitative agreement with experiments by Wernsdorfer and Sessoli. The particular case H z =0 was already obtained by Garg by means of path integrals. The diabolic values of are in agreement with numerical results but, as already noticed by Wernsdorfer and Sessoli, they disagree with the experimental ones. This may be an effect of higher order anisotropy terms, which is briefly addressed in the conclusion. Received 17 May 2000
Keywords:PACS  75  45  +j Macroscopic quantum phenomena in magnetic systems - 75  50  Xx Molecular magnets - 61  46  +w Clusters  nanoparticles            and nanocrystalline materials
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