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Kinetic Modeling of Plasma Methane Conversion Using Gliding Arc
引用本文:AntoniusIndarto Jae-WookChoi HwaungLee HyungKeunSong. Kinetic Modeling of Plasma Methane Conversion Using Gliding Arc[J]. 天然气化学杂志, 2005, 14(1): 13-21
作者姓名:AntoniusIndarto Jae-WookChoi HwaungLee HyungKeunSong
作者单位:CleanTechnologyResearchCenter,KoreaInstituteofScience&Technology,P.O.Box131,Cheongryang,Seoul130-650,Korea
摘    要:Plasma methane (CH4) conversion in gliding arc discharge was examined. The result data of experiments regarding the performance of gliding arc discharge were presented in this paper. A simulation which is consisted some chemical kinetic mechanisms has been provided to analyze and describe the plasma process. The effect of total gas flow rate and input frequency refers to power consumption have been studied to evaluate the performance of gliding arc plasma system and the reaction mechanism of decomposition.Experiment results indicated that the maximum conversion of CH4 reached 50% at the total gas flow rate of 1 L/min. The plasma reaction was occurred at the atmospheric pressure and the main products were C (solid), hydrogen, and acetylene (C2H2). The plasma reaction of methane conversion was exothermic reaction which increased the product stream temperature around 30~50℃.

关 键 词:等离子体 甲烷转化 反应机理 滑动电弧光 反应动力学 热力学计算

Kinetic Modeling of Plasma Methane Conversion Using Gliding Arc
Antonius Indarto,Jae-Wook Choi,Hwaung Lee,Hyung Keun Song. Kinetic Modeling of Plasma Methane Conversion Using Gliding Arc[J]. Journal of Natural Gas Chemistry, 2005, 14(1): 13-21
Authors:Antonius Indarto  Jae-Wook Choi  Hwaung Lee  Hyung Keun Song
Affiliation:Clean Technology Research Center, Korea Institute of Science & Technology, P.O. Box 131, Cheongryang, Seoul 130-650, Korea
Abstract:Plasma methane (CH4) conversion in gliding arc discharge was examined. The result data of experiments regarding the performance of gliding arc discharge were presented in this paper. A simulation which is consisted some chemical kinetic mechanisms has been provided to analyze and describe the plasma process. The effect of total gas flow rate and input frequency refers to power consumption have been studied to evaluate the performance of gliding arc plasma system and the reaction mechanism of decomposition.Experiment results indicated that the maximum conversion of CH4 reached 50% at the total gas flow rate of 1 L/min. The plasma reaction was occurred at the atmospheric pressure and the main products were C (solid), hydrogen, and acetylene (C2H2). The plasma reaction of methane conversion was exothermic reaction which increased the product stream temperature around 30-50 ℃.
Keywords:plasma  gliding arc  methane conversion  reaction mechanism
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