Dynamical theory of spectroscopy with femtosecond pulse excitation |
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Authors: | Jing Lu Soo-ying Lee Kangnian Fan |
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Institution: | 1. Department of Chemistry, Fudan University, 200433, Shanghai, China 2. Department of Chemistry, National University of Singapore, 119260, Singapore, Singapore
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Abstract: | The dynamical theory of spectroscopy with femtosecond pulse excitation is applied to a direct dissociation process. In the ultrashort pulse case, the fluorescence-like emission peak occurs in Raman scattering as the incident frequency is tuned near resonance. All properties of the spectroscopy can be explained by the correlation function. |
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