Many body contributions to the electronic structure of nickel

The full temperature-dependence of the electronic quasiparticle properties of ferromagnetic Ni is investigated by use of a theoretical model, which takes into account all intraatomic interactions in thed-band complex. After introduction of effective spin operators the model-Hamiltonian consists of a one-particle term, an intraband-interaction of Hubbardtype, and an interband-exchange as in thes-f (ord-f model. The one-particle energies are taken from a realistic bandstructure calculation in order to incorporate approximately all those interactions, which are not directly covered by our model. The model contains two parameters, the intraband couplingU and the interband exchangeJ. ChoosingU=6 eV,J=0.4 eV and applying a Green-function technique we get results in almost quantitative agreement with the experiment:T _c=635 K,m(T=0)=0.56 _B , Curie-Weiss behaviour of the static susceptibility, satellite peak with temperature-dependent spinpolarization some 6 eV below the chemical potential , exchange splittings atT=0 of order 0.2–0.35 eV. The full temperature-dependencies of the electronic selfenergy, the one-particle spectral density, the quasiparticle density of states, and the quasiparticle bandstructure for two high symmetry directions are derived and discussed.