| 光电化学催化中的富勒烯基材料：机理及应用 |
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| 引用本文： | 程源晟,蔡号东,凌敏,宋超,魏先文. 光电化学催化中的富勒烯基材料：机理及应用[J]. 无机化学学报, 2020, 36(6): 1014-1034 |
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| 作者姓名： | 程源晟 蔡号东 凌敏 宋超 魏先文 |
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| 作者单位： | 安徽工业大学化学与化工学院, 材料科学与工程研究院, 煤清洁转化与高值化利用安徽省重点实验室, 马鞍山 243002;安徽师范大学化学与材料科学学院, 功能分子固体教育部重点实验室, 芜湖 241000;广西科学院广西红树林研究中心, 北海 536000;1 安徽工业大学化学与化工学院, 材料科学与工程研究院, 煤清洁转化与高值化利用安徽省重点实验室, 马鞍山 243002;安徽工业大学化学与化工学院, 材料科学与工程研究院, 煤清洁转化与高值化利用安徽省重点实验室, 马鞍山 243002 |
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| 基金项目： | 国家自然科学基金（No.21771003）资助项目。 |
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| 摘 要： | 光催化和电化学催化在现代清洁能源转化中发挥了无可替代的作用。[60]富勒烯(C_(60))材料因其独特的结构与性能而被广泛用于各类光电催化剂的开发中,并取得了令人瞩目的成果。我们简介了C_(60)的基本性质以及富勒烯基(包括C_(60)笼外衍生物和衍生碳材料)光电催化剂的制备方法,综述了C_(60)及其衍生材料在光催化和电化学催化领域中的研究进展,就其在光电化学催化应用中所起到的主要作用、工作机理以及优化策略进行了讨论。并对C_(60)基催化剂发展中的主要问题与挑战进行了总结和展望。
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| 关 键 词： | 富勒烯 能量转换 多相催化 光化学 电化学 绿色化学 |
| 收稿时间： | 2020-03-09 |
| 修稿时间： | 2020-04-02 |
Fullerene-Based Materials in Photocatalysis and Electrochemical Catalysis: Fundamentals and Applications |
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| CHENG Yuan-Sheng,CAI Hao-Dong,LING Min,SONG Chao,WEI Xian-Wen. Fullerene-Based Materials in Photocatalysis and Electrochemical Catalysis: Fundamentals and Applications[J]. Chinese Journal of Inorganic Chemistry, 2020, 36(6): 1014-1034 |
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| Authors: | CHENG Yuan-Sheng CAI Hao-Dong LING Min SONG Chao WEI Xian-Wen |
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| Affiliation: | School of Chemistry and Chemical Engineering, Institute of Materials Sciences and Engineering, Anhui Province Key Laboratory of Coal Clean Conversion and High Valued Utilization, Anhui University of Technology, Maanshan, Anhui 243002, China;College of Chemistry and Materials Science, the Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Normal University, Wuhu, Anhui 241000, China;Guangxi Mangrove Research Center, Guangxi Academy of Sciences, Beihai, Guangxi 536000, China; 1 School of Chemistry and Chemical Engineering, Institute of Materials Sciences and Engineering, Anhui Province Key Laboratory of Coal Clean Conversion and High Valued Utilization, Anhui University of Technology, Maanshan, Anhui 243002, China;School of Chemistry and Chemical Engineering, Institute of Materials Sciences and Engineering, Anhui Province Key Laboratory of Coal Clean Conversion and High Valued Utilization, Anhui University of Technology, Maanshan, Anhui 243002, China |
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| Abstract: | Photocatalysis and electrochemical catalysis play an irreplaceable role in modern clean energy conversion. [60]Fullerene (C60) is widely used in novel catalysts designing because of its unique structures and properties, and has made satisfactory results. Herein, we have briefly introduced the basic properties and synthesis strategies for C60 (including C60 derivatives and C60 derived carbon materials) based catalysts. Providing a comprehensive overview of currently researches about the applications of C60 and C60 derives in photocatalysis and electrochemical catalysis. Furthermore, the functions, action mechanisms and the strategies of performance improvement for C60 based catalysts are systematically discussed. Some key issues and challenges in the development of C60 based catalysts are also proposed. |
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| Keywords: | fullerenes energy conversion heterogeneous catalysis photochemistry electrochemistry green chemistry |
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