Mori-Zwanzig memory analysis in single-molecule spectroscopy |
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Authors: | Schmitt Daniel T Schulz Michael Reineker Peter |
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Affiliation: | Theoretische Physik, Universit?t Ulm, D-89069 Ulm, Germany. |
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Abstract: | We study the dynamical behavior of the Rhodospirillum molischianum LH2 complex based on intensity time series obtained from single-molecule spectroscopy experiments. This is achieved by reconstructing the memory function describing the time-dependent fluctuations of the excited states. We conclude that the apparent stochastic evolution of the dynamics is controlled by at least two different non-Markovian main processes. |
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