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Hydrogen-bonding 2D metal-organic solids as highly robust and efficient heterogeneous green catalysts for Biginelli reaction |
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| Authors: | Li Peng Regati Sridhar Butcher Raymond J Arman Hadi D Chen Zhenxia Xiang Shengchang Chen Banglin Zhao Cong-Gui |
| Affiliation: | a Department of Chemistry, University of Texas at San Antonio, One UTSA Circle, San Antonio, TX 78249-0698, United States b Department of Chemistry, Howard University, Washington, DC 20059, United States c Department of Chemistry, Fudan University, Shanghai 200433, PR China |
| Abstract: | Two new Zn(II) and Cd(II) MOFs have been synthesized. These MOFs have been applied as heterogeneous catalysts for the green synthesis of a variety of dihydropyrimidinone derivatives through the Biginelli reaction and the desired products were obtained in high yields with short reaction time under mild solvent-free conditions. Moreover, the MOF catalysts may be readily recovered after the reaction and reused for many cycles. |
| Keywords: | Metal-organic framework Biginelli reaction Heterogeneous catalyst Solvent-free conditions Green reactions |
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