| Constructing a coplanar heterojunction through enhanced π-π conjugation in g-C3N4 for efficient solar-driven water splitting |
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| 作者姓名： | Zihao Chen Ben Chong Nathan Wells Guidong Yang Lianzhou Wang |
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| 作者单位： | 1. XJTU-Oxford International Joint Laboratory for Catalysis, School of Chemical Engineering and Technology, Xi'an Jiaotong University;2. School of Chemical Engineering and Australian Institute for Bioengineering and Nanotechnology, the University of Queensland |
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| 基金项目： | financially supported by the National Natural Science Foundation of China (Nos. U1862105, 22078256);;Natural Science Basic Research Plan in Shaanxi Province of China (Nos. 2017JZ001, 2018KJXX-008);;Fundamental Research Funds for the Central Universities (No. cxtd2017004);;K.C. Wong Education Foundation, Hong Kong, China;;financial support from Australian Research Council are appreciated; |
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| 摘 要： | Adjusting the electronic structure of graphitic carbon nitride（g-C3N4） photocatalyst through π-π conjugation is an effective method to achieve efficient photogenerated carrier separation. One key challenge ofπ-π conjugation control is to tune the degree of such conjugation without destroying the g-C3N4structure. Herein we report a conceptual design that achieves a coplanar heterojunction by enhancing theπ-π conjugation via the doping of crystalline g-C...
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| 收稿时间： | 2021-07-28 |
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