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Rapid activation product separations from fission products and soil matrixes
Authors:Bennett  Kevin T.  Kozimor  Stosh A.  Manard  Benjamin T.  Mocko  Veronika  Pacheco  Susan D.  Schake  Ann R.  Wu  Ruilian  Olson  Angela C.
Affiliation:1.Los Alamos National Laboratory, P.O. Box 1663, Los Alamos, NM, 87545, USA
;2.Oak Ridge National Laboratory, 1 Bethel Valley Rd, Oak Ridge, TN, 37830, USA
;
Abstract:

A rapid method for the separation and qualitative analysis of several neutron activation products (198Au, 192Ir, 72Ga, 51Cr, 191/195m/197Pt, 54Mn, 57Co, and 59Fe) from fission products and soil matrixes has been developed. Analytes were isolated within 20 h using ion exchange chromatography. After separation, the activation products were characterized by γ-spectroscopy and inductively coupled plasma-optical emission spectroscopy. Validation experiments demonstrated versatility of the method, showing that the activation products could be isolated from fresh fission products and other contaminants associated with complex soil matrixes.

Keywords:
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