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Synergistic effect of polylactic acid(PLA) and Poly(butylene succinate-co-adipate) (PBSA) based sustainable,reactive, super toughened eco-composite blown films for flexible packaging applications
Institution:1. Department of Chemical and Materials Engineering, Chang Gung University, Tao-Yuan, 333, Taiwan;2. Department of General Dentistry, Chang Gung Memoral Hospital, Tao-Yuan, 333, Taiwan;1. Federal University of São Carlos, Graduate Program in Materials Science and Engineering, Rod. Washington Luiz, Km 235, São Carlos, São Paulo, 13565-905, Brazil;2. Federal University of São Carlos, Department of Materials Engineering, Rod. Washington Luiz, Km 235, São Carlos, São Paulo, 13565-905, Brazil;3. Luxembourg Institute of Science and Technology, Materials Research and Technology Department, 5 Avenue des Hauts-Fourneaux, L-4362, Esch-sur-Alzette, Luxembourg;1. Institute for Polymers, Composites and Biomaterials—National Research Council, Via Campi Flegrei 34, Pozzuoli, 80078 Naples, Italy;2. Department of Chemical, Materials and Production Engineering, University of Naples, Piazzale Tecchio 80, 80125 Napoli, Italy;3. Department of Materials Engineering, Faculty of Technology, University of Amazonas, Av. General Rodrigo Octávio Jordão Ramos, 6200, Coroado I, 69077-000 Manaus, Brasil
Abstract:Polylactic acid (PLA)/poly (butylene succinate-co-adipate) (PBSA) based blend films at variable compositions and fixed weight percentage of Epoxy functionalized styrene acrylate (ESA) were prepared using a single step blending process, followed by blown film extrusion process. The morphological studies revealed proper interaction between polymers by the interaction of chain extender (ESA) subsequently improved the mechanical properties of the prepared blown films. Similarly, the blend films showed a decrease in oxygen transmission rate (OTR) and water vapor transmission rate (WVTR) in the order of 60% and 14% as compared with VPLA film. The optical and antislip properties of the blend films also increased considerably. The thermal analysis of the blend films depicted marginal enhancement in the stability of PLA along with heterogeneous nucleation effect in PLA matrix due to the presence of ESA and PBSA.
Keywords:PLA  PBSA  ESA  OTR  WVTR  Antislip property
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