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可用于环境修复的半导体光催化剂及其改性策略研究进展
引用本文:王慧杰,李鑫,赵小雪,李春岩,宋相海,张鹏,霍鹏伟. 可用于环境修复的半导体光催化剂及其改性策略研究进展[J]. 催化学报, 2022, 0(2): 178-214. DOI: 10.1016/S1872-2067(21)63910-4
作者姓名:王慧杰  李鑫  赵小雪  李春岩  宋相海  张鹏  霍鹏伟
作者单位:江苏大学化学化工学院, 绿色化学与化工技术研究院, 江苏镇江212013;江苏大学流体机械工程与技术研究中心, 江苏镇江212013;郑州大学材料科学与工程学院, 河南郑州450001;华南农业大学生物质工程研究院, 农业部能源植物资源与利用重点实验室, 广东广州510642
基金项目:国家自然科学基金(22078131,21776117).
摘    要:多相光催化技术作为一种直接利用太阳光降解多种污染物的先进氧化工艺在环境修复领域的研究中引起了广泛关注.在多相光催化过程中,半导体材料在太阳光的激发下,其强大的氧化/还原能力可快速高效降解各种污染物.研究者通常根据环境中污染物的状态和种类选择合适的半导体材料及修饰策略,构建高效多相光催化体系,探究光催化材料在环境修复中的...

关 键 词:污染物  多相光催化  环境修复  半导体  修饰策略

A review on heterogeneous photocatalysis for environmental remediation: From semiconductors to modification strategies
Huijie Wang,Xin Li,Xiaoxue Zhao,Chunyan Li,Xianghai Song,Peng Zhang,Pengwei Huo. A review on heterogeneous photocatalysis for environmental remediation: From semiconductors to modification strategies[J]. Chinese Journal of Catalysis, 2022, 0(2): 178-214. DOI: 10.1016/S1872-2067(21)63910-4
Authors:Huijie Wang  Xin Li  Xiaoxue Zhao  Chunyan Li  Xianghai Song  Peng Zhang  Pengwei Huo
Affiliation:(Institute of Green Chemistry and Chemical Technology,School of Chemistry and Chemical Engineering,Jiangsu University,Zhenjiang 212013,Jiangsu,China;Research Center of Fluid Machinery Engineering and Technology,Jiangsu University,Zhenjiang 212013,Jiangsu,China;School of Materials Science and Engineering,Zhengzhou University,Zhengzhou 450001,Henan,China;Institute of Biomass Engineering,Key Laboratory of Energy Plants Resource and Utilization,Ministry of Agriculture and Rural Affairs,South China Agricultural University,Guangzhou 510642,China)
Abstract:Heterogeneous photocatalysis, an advanced oxidation process, has garnered extensive attention in the field of environmental remediation because it involves the direct utilization of solar energy for the removal of numerous pollutants. However, the application of heterogeneous photocatalysis in environmental remediation has not achieved the expected consequences due to enormous chal-lenges such as low photocatalytic efficiencies and high costs of heterogeneous photocatalysts in large-scale practical applications. Furthermore, pollutants in the natural environment, including water, air, and solid phases, are diverse and complex. Therefore, extensive efforts should be made to better understand and apply heterogeneous photocatalysis for environmental remediation. Herein, the fundamentals of heterogeneous photocatalysis for environmental remediation are introduced. Then, potential semiconductors and their modification strategies for environmental photocatalysis are systematically presented. Finally, conclusions and prospects are briefly summarized, and the direction for the future development of environmental photocatalysis is explored. This review may provide reference directions toward understanding, researching, and designing photocatalytic re-mediation systems for various environmental pollutants.
Keywords:Pollutant  Heterogeneous photocatalysis  Environmental remediation  Semiconductor  Modification strategy
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