Abstract: | Nonlinear plasmonic metasurfaces are compatible with complementary metal oxide semiconductor technology and highly promising for on-chip optical switching and modulations and nanoscale frequency conversions. However, the low nonlinearoptical response of metasurface devices limits their practical applications. To circumvent this constraint, we propose the design of a nanocavity plasmonic metasurface, in which the strong light localization in the nanocavity can be used to boost the efficiency of second-harmonic generation. Compared with the single-layer counterpart, experimental results show that the intensity of the second-harmonic waves in the nanocavity metasurface is enhanced by ~790 times. The proposed nanocavity plasmonic metasurfaces in this work may open new routes for developing highly efficient nonlinear metacrystals for on-chip nonlinear sources,nonlinear image encryption, information processing, and so on. |