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A low-temperature electron diffraction study of structural disorder and its relationship to the Kondo effect in ThAsSe
Authors:RL Withers  R Vincent
Institution:
  • a Research School of Chemistry, Australian National University, Canberra ACT 0200, Australia
  • b H.H.Wills Physics Laboratory, University of Bristol, Bristol BS8 1TL, UK
  • c Institute for Semiconductor Physics and Optics, Technical University Braunschweig, D-38106 Braunschweig, Germany
  • Abstract:A low-temperature electron diffraction study has been carried out on ThAsSe to search for evidence of structural disorder associated with the low-temperature non-magnetic Kondo effect. A highly structured and extremely complex characteristic diffuse intensity distribution has been observed at low temperature and interpreted in terms of a gradual charge density wave type phase transition upon lowering of temperature involving disordered As-As dimerization within (001) planes. Plausible models of the proposed As-As dimerization have been obtained using a group theoretical approach.
    Keywords:Kondo effect  As dimerization  Charge density wave  Transmission electron microscopy  Incommensurately modulated
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