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Spin lattice coupling in multiferroic hexagonal YMnO3
Authors:Sylvain Petit  Stéphane Pailhès  Xavier Fabrèges  Martine Hennion  Fernande Moussa  Loreynne Pinsard  Louis-Pierre Regnault  Alexander Ivanov
Affiliation:(1) LLB, CEA-CNRS (UMR 12), CE-Saclay, F-91190 Gif sur Yvette, France;(2) Laboratoire de Chimie des Solides, URA 446 CNRS, Université Paris-Sud, Orsay, France;(3) CEA-Grenoble, DRFMC-SPSMS-MDN, 17 rue des Martyrs, F-38054 Grenoble, France;(4) Institut Laue Langevin, 6, rue Jules Horowitz, BP 156, F-38042 Grenoble, France
Abstract:Aiming to shed light on the possible existence of hybrid phonon-magnon excitations in multiferroic manganites, neutron scattering measurements have been undertaken at LLB and ILL on the particular case of hexagonal YMnO3. Our experiments focused on a transverse acoustic phonon mode polarized along the ferroelectric axis. The neutron data show that below the magnetic transition, this particular phonon mode splits in two different branches. The upper branch is found to coincide with a spin wave mode. This manifestation of a strong spin-lattice coupling is discussed in terms of a possible hybridization between the two types of elementary excitations, the phonon and magnons.
Keywords:Multiferroic  manganites  spin phonon hybridization  inelastic neutron scattering
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