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Evolution of the initially ordered structure in a magnetic fluid film during a thermal cycle
Authors:Y?H?Ke  S?Y?Yang  Email author" target="_blank">H?E?HorngEmail author  Chin-Yih?Hong  H?C?Yang
Institution:(1) Department of Physics, National Taiwan Normal University, 116 Taipei, Taiwan;(2) Institute of Electro-optical Science and Technology, National Taiwan Normal University, 116 Taipei, Taiwan;(3) Department of Mechanical and Automation Engineering, Da-Yeh University, 515 Changhwa, Taiwan;(4) Department of Physics, National Taiwan University, 106 Taipei, Taiwan
Abstract:A hexagonal ordered structure of magnetic columns, which results from an agglomeration of magnetic particles, is obtained in a magnetic fluid film when a magnetic field is applied perpendicularly to the film surface. The evolution of the initially ordered structure in the magnetic fluid film during the heating and cooling process is investigated under a given magnetic field. For the heating process, the columns remain unchanged until the temperature exceeds a critical temperature. As the temperature is further increased, column particles start to disperse into the liquid carrier. As a result, portions of columns disappear. As the temperature continue to rise, the ordered structure changes to a disordered column state, or even a monodispersed state. On the other hand, when the temperature is lowered, the magnetic particles in the carrier condense out of solution and finally an ordered structure of columns is achieved. However, this structural evolution during a thermal cycle is irreversible.Received: 28 August 2004, Published online: 21 October 2004PACS: 75.50.Mm Magnetic liquids - 64.75. + g Solubility, segregation, and mixing; phase separation - 68.60.Dv Thermal stability; thermal effects
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