Fractional revivals in the rovibrational motion of I2 |
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Authors: | Lohmüller T Engel V Beswick J A Meier C |
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Institution: | Institut für Physikalische Chemie, Universit?t Würzburg, Am Hubland, D-97074 Würzburg, Germany. |
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Abstract: | Motivated by pump-probe experiments of I(2) in a room-temperature sample, the detection of fractional revivals is investigated using full-dimensional quantum wave packet calculations. It is shown that the structures observed in the pump-probe signal depend sensitively on the probe parameters employed and that the observed signal reflects a particular phase effect between fractional revivals. |
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