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Thermal energy collisions between metastable Ne?(2p 53s,3 P 0, 2) and H2(X,1Σ g + )
Authors:J Robert  V Bo?varski  B Stern  J Reinhardt  J Baudon
Institution:1. Laboratoire de Physique des Lasers, Associé au CNRS, Université Paris-Nord, Villetaneuse, France
Abstract:A crossed beam experiment is used to investigate the Ne*(2p 5 3s,3 P 0, 2) ? H2(1Σ g + ) collision at thermal energy (67 meV). The H2 beam is supersonic, the Ne* beam is thermal. Different collision processes have been analyzed separately by means of a double chopping technique combined with a time of flight measurement. Ions produced by Penning effect and chemi-ionization have been separated from scattered metastable atoms by an accelerating electric field small enough to preserve a reasonable angular resolution: δ?(ions)=±5.5°, δ?(Ne*)=±1°, which allows a determination of differential cross sections. The attenuation method, combined with an absolute measurement of the total H2 flux, has been used to measure the total cross section: σ t =940±220a 0 2 . Differential cross sections have been obtained, in arbitrary but unique unit, for the following processes: (1) elastic collisions, for a mixture (1:3) of para- and ortho-hydrogen; (2) rotationally inelastic collisions:J=0→2; (3) Penning ionization resulting into H 2 + ions; (4) chemiionization yielding NeH+ ions.
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