Multiple nuclear spin echo in thin polycrystalline ferromagnetic films

The formation of multiple nuclear spin echo signals has been studied in thin ferromagnetic polycrystalline films of 3d-metals and their alloys with induced anisotropy at temperatures between 2.2 and 300 K using two-pulse and three-pulse excitation. A method is proposed for the experimental determination of the contributions made by different mechanisms to the formation of spin-echo signals in magnets with strongly inhomogeneous Zeeman and quadrupole interactions. It is shown that in ferromagnets with a high rf field gain at the nucleus, the frequency modulation mechanism has a substantial influence in observations of nuclear spin-echo signals at nuclei with a high magnetic moment, even at liquid-helium temperatures. Fiz. Tverd. Tela (St. Petersburg) 40, 1056–1061 (June 1998)