Measurements of mid-stratospheric formaldehyde from the Odin/SMR instrument |
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Authors: | P Ricaud D Alexandre E Le Flochmoën G Berthet D Murtagh |
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Institution: | a Laboratoire d’Aérologie, CNRS/Université de Toulouse III, 14, Avenue Edouard Belin, 31400, Toulouse, France b Laboratoire de Physique et de Chimie de l’Environnement, CNRS, 3A, Avenue de la Recherche Scientifique, 45071 Orléans Cedex 2, France c Service d’Aéronomie, CNRS, Université Pierre et Marie Curie, 4 Place Jussieu, 75252 Paris Cedex 05, France d Department of Radio and Space Science, Chalmers University of Technology, 412 96 Göteborg, Sweden |
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Abstract: | Measurements of mid-stratospheric formaldehyde (H2CO) have been obtained from the limb-viewing sub-millimeter radiometer (SMR) instrument aboard the Odin satellite. The analysis is based upon the only weak (808→707) rotational transition line of H2CO that can be measured by Odin/SMR at 576.7083150 GHz in the band dedicated to the measurement of carbon monoxide (CO). The signal-to-noise ratio is increased by averaging about 1000 spectra within 2-km width vertical layers in the stratosphere over periods from 1 to 7 days and within 3 latitude bands: Southern Hemisphere (90°S-45°S), tropics (30°S-30°N), and Northern Hemisphere (45°N-90°N). The faint H2CO line can then be retrieved using the standard scientific ground-segment developed for the Odin/SMR measurements. The mid-stratospheric H2CO shows maxima in the tropics for every period considered (January 2006, February 2005, March 2005, and September 2005). The spring-time extra-tropical mid-stratospheric H2CO is more intense than the fall-time extra-tropical amounts. The simulations from the three-dimensional chemical-transport model Reprobus satisfactorily show these general features. |
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Keywords: | Radiative transfer Spectroscopy Inversion Formaldehyde Remote sensing Satellite Stratosphere |
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