Magnetic structure of iron-doped UPd2Ge2

Neutron diffraction investigations have shown that a 2% substitution Fe atoms for Pd radically alters the magnetic structure of UPd²Ge². If the magnetic structure in the undoped compound at T>50 K consists of a longitudinal spin density wave (LSDW) with “square” modulation, then in polycrystalline U(Pd^0.98Fe^0.02)²Ge² a “simple” antiferromagnetic (AF) phase is observed below 65 K and a sinusoidally modulated LSDW-AF phase is observed between 65 K and the Neel temperature T ^N =135 K. In the interval 65> T>135 K the magnetic cell is incommensurate with the crystal cell, with the exception of the point T=93 K, where the wave vector of the magnetic structure passes through a “commensurate” value equal to 0.75. Below T ^N the magnetic moments of the uranium atoms are always parallel to the tetragonal axis c of the unit cell. Pis’ma Zh. éksp. Teor. Fiz. 66, No. 9, 615–619 (10 November 1997)