外场作用下BaF分子发射光子累积量及等待时间分布的研究

利用产生函数方法对BaF分子在激光场与射频场作用下发射光子的累积量及等待时间分布进行了研究. 累积量κ₁ 和κ₂ 表明在固有偶极和射频场的作用下, 系统表现出外场辅助吸收的现象, 即当Δ₁=nω_rf时, 系统存在吸收峰. 二阶、三阶等待时间分布呈现出明显的振荡现象.

Cumulants and waitingtime distribution of the photon emission from driven BaF molecule

In this paper, we consider a single BaF molecule driven by an external field. When the symmetry is broken, the states of the BaF molecule demonstrate the permanent dipole moments. An external laser field to excite BaF molecule transition from its ground state to its excited state, and a radio frequency field couple with the permanent dipole moment of the BaF. The first order and second order cumulants of the emission photons and the waiting time distribution are studied via the recently developed generating function approach, which is very convenient to study the counting statistics and the corresponding probability distributions. The results demonstrate that the radio frequency field could help the BaF molecule to absorb photons from the driving field. The second and third order waiting time distributions oscillate with the evolution time, which reflects the states oscillating with the external radio frequency field.