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Fabrication and characterization of high performance cathode supported small-scale SOFC for intermediate temperature operation
Authors:Toshiaki Yamaguchi   Sota Shimizu   Toshio Suzuki   Yoshinobu Fujishiro  Masanobu Awano
Affiliation:aNational Institute of Advanced Industrial Science and Technology (AIST), 2266-98 Anagahora, Shimo-shidami, Moriyama-ku, Nagoya, Aichi 463-8563, Japan;bFine Ceramics Research Association (FCRA), Shimo-shidami, Moriyama-ku, Nagoya 463-8561, Japan
Abstract:A high performance small-scale solid oxide fuel cell supported by a microtubular cathode was successfully developed via the extrusion of a (La0.8Sr0.2)0.97MnO3 cathode support and subsequent surface coating with a (La0.8Sr0.2)0.97MnO3–Ce0.9Gd0.1O1.95 activation layer followed by Sc2O3-doped ZrO2 electrolyte and NiO–Ce0.9Gd0.1O1.95 anode slurries. The cell was electrochemically evaluated in a humidified hydrogen (3% H2O) atmosphere, and exhibited a stable open circuit voltage above 1.05 V in the temperature range from 550 to 750 °C. Maximum power densities of 46.5, 163.2 and 452.8 mW cm−2 were generated at 550, 650 and 750 °C, respectively. The results indicate the realization of a stable and high performance cathode-supported micro SOFC.
Keywords:Micro SOFC   Tubular LSM support   Wet coating   Activation layer   ScSZ electrolyte
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