Signatures of dynamical heterogeneity in the structure of glassy free-energy minima |
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Authors: | Chaudhuri Pinaki Karmakar Smarajit Dasgupta Chandan |
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Affiliation: | Department of Physics, Indian Institute of Science, Bangalore 560012, India. |
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Abstract: | From numerical minimization of a model free-energy functional for a system of hard spheres, we show that the width of the local peaks of the time-averaged density field at a glassy free-energy minimum exhibits large spatial variation, similar to that of the "local Debye-Waller factor" in simulations of dynamical heterogeneity. Molecular dynamics simulations starting from a particle configuration generated from the density distribution at a glassy free-energy minimum show similar spatial heterogeneity in the degree of localization, implying a direct connection between dynamical heterogeneity and the structure of glassy free-energy minima. |
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