Threshold laws in delayed emission: an experimental approach |
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Authors: | B Climen F Pagliarulo A Ollagnier B Baguenard B Concina M A Lebeault F Lépine C Bordas |
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Institution: | (1) Laboratoire de Spectrométrie Ionique et Moléculaire, UMR CNRS 5579, Université Lyon 1, 69622 Villeurbanne, France |
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Abstract: | Delayed emission is a common decay process for very excited complex systems
where the excitation energy is, to a large extent, statistically distributed
over all accessible degrees of freedom. A rich variety of delayed decay
processes is found in complex molecules and clusters such as thermionic
emission, evaporation of heavy fragments or blackbody radiation. In this
article, we present the general threshold laws that govern the kinetic
energy spectrum of matter particles (electrons or fragments) ejected from
spherically symmetric species in such processes, and we illustrate these
laws by experimental results obtained in photoelectron and photoion
spectroscopy. Deviations from simple laws for non spherical species are also
evidenced. |
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Keywords: | 36 40 -c Atomic and molecular clusters 36 40 Qv Stability and fragmentation of clusters 33 60 Cv Ultraviolet and vacuum ultraviolet photoelectron spectra |
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