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Few-Layer Fullerene Network for Photocatalytic Pure Water Splitting into H2 and H2O2
Authors:Taotao Wang  Li Zhang  Jinbao Wu  Prof Muqing Chen  Prof Shangfeng Yang  Prof Yalin Lu  Prof Pingwu Du
Institution:1. Key Laboratory of Precision and Intelligent Chemistry, Anhui Laboratory of Advanced Photon Science and Technology, Department of Materials Science and Engineering, University of Science and Technology of China, 96 Jinzhai Road, Hefei, Anhui Province, 230026 P. R. China

School of Materials Science and Engineering, Dongguan University of Technology, Dongguan, Guangdong Province, 523808 P. R. China;2. Key Laboratory of Precision and Intelligent Chemistry, Anhui Laboratory of Advanced Photon Science and Technology, Department of Materials Science and Engineering, University of Science and Technology of China, 96 Jinzhai Road, Hefei, Anhui Province, 230026 P. R. China;3. School of Materials Science and Engineering, Dongguan University of Technology, Dongguan, Guangdong Province, 523808 P. R. China

Abstract:A few-layer fullerene network possesses several advantageous characteristics, including a large surface area, abundant active sites, high charge mobility, and an appropriate band gap and band edge for solar water splitting. Herein, we report for the first time that the few-layer fullerene network shows interesting photocatalytic performance in pure water splitting into H2 and H2O2 in the absence of any sacrificial reagents. Under optimal conditions, the H2 and H2O2 evolution rates can reach 91 and 116 μmol g?1 h?1, respectively, with good stability. This work demonstrates the novel application of the few-layer fullerene network in the field of energy conversion.
Keywords:Fullerene  Hydrogen  Hydrogen Peroxide  Nanosheet  Solar Water Splitting
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