Coherent manipulation of electron spins in the {Cu3} spin triangle complex impregnated in nanoporous silicon |
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Authors: | Choi K-Y Wang Z Nojiri H van Tol J Kumar P Lemmens P Bassil B S Kortz U Dalal N S |
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Affiliation: | Department of Physics, Chung-Ang University, Seoul, Republic of Korea. kchoi@cau.ac.kr |
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Abstract: | We report on coherent manipulation of electron spins in an antiferromagnetically coupled spin triangle {Cu3-X} (X=As, Sb) impregnated in freestanding nanoporous silicon (NS) by using 240 GHz microwave pulses. Rabi oscillations are observed and the spin coherence time is found to be T(2)=1066 ns at 1.5 K. This demonstrates that the {Cu3-X}:NS hybrid material provides a promising scheme for implementing spin-based quantum gates. By measuring the spin relaxation times of samples with different symmetries and environments we give evidence that a spin chirality is the main decoherence source of spin triangle molecules. |
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