Investigation of the structure of the reaction center in photosynthetic systems by optical detection of triplet state magnetic resonance |
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Authors: | Richard H. Clarke Robert E. Connors Harry A. Frank Jeffrey C. Hoch |
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Affiliation: | Department of Chemistry, Boston University, Boston, Massachusetts 02215, USA |
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Abstract: | Properties expected of the triplet state of a pair of interacting pigment molecules in photosynthetic systems are described in terms of the triplet state properties of the monomer pigment. The triplet state zero-field splittings and intersystem crossing rate constants measured in isolated chlorophylls and the same properties measured in vivo are utilized to elucidate the geometry of the eraction center in photosynthetic systems. |
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