Enantiocontrolled total syntheses of breviones A, B, and C |
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| Authors: | Yokoe Hiromasa Mitsuhashi Chika Matsuoka Yoko Yoshimura Tomoyuki Yoshida Masahiro Shishido Kozo |
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| Institution: | Graduate School of Pharmaceutical Sciences, The University of Tokushima, 1-78-1 Sho-machi, Tokushima 770-8505, Japan. |
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| Abstract: | Enantiocontrolled total syntheses of the breviones A, B, and C have been accomplished using a highly diastereoselective oxidative coupling of an α-pyrone with a tricyclic diene prepared from an optically pure Wieland-Miescher ketone derivative through the 7-endo-trig mode of acyl radical cyclization. |
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